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Stars

Nuclei

Laboratory

Nuclear

Astrophysics

at CERN n_TOF

Expression of Interest for the CERN 20-year Roadmap of Non-Collider Physics

C. Domingo-Pardo, C. Lederer-Woods

on behalf of the n_TOF Collaboration

INTC Meeting · CERN, Geneva · 4 November 2026

CERN-INTC-2026-014 · INTC-EOI-002

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Nuclear

Astrophysics

at CERN n_TOF

Expression of Interest for the CERN 20-year Roadmap of Non-Collider Physics

C. Domingo-Pardo, C. Lederer-Woods

on behalf of the n_TOF Collaboration

INTC Meeting · CERN, Geneva · 4 November 2026

CERN-INTC-2026-014 · INTC-EOI-002

  1. Scientific Motivation & Impact
  2. Programme Definition
  3. Why at CERN: Uniqueness & Synergies
  4. Timeline
  5. Summary

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3

  • Sites and evolution: which sources make the heavy elements, and how did their contributions change over Galactic history?
  • Stellar conditions: what are the temperatures and neutron densities of the s-, i- and r-processes, and how much does each contribute?
  • Presolar grains and stellar spectra: what produces their peculiar abundance patterns?
  • Radioactivities and chronometers: how do neutron-induced reactions set their abundances?
  • Beyond Pb/Bi: how does nucleosynthesis proceed, and what is the role of fission?

​

Open questions on the origin of the heavy elements

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4

(I) Stellar models and presolar grains

  • Re-measure the stable isotopes with MACS uncertainties >5% to ≤5%
    • Stations: EAR1, EAR2, NEAR

1xEoIs: EoI n_TOF facility upgrades, M.Bacak et al.

​

​

Programme: three physics pillars and the stations that serve them

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5

(I) Stellar models and presolar grains

  • Re-measure the stable isotopes with MACS uncertainties >5% to ≤5%
    • Stations: EAR1, EAR2, NEAR

1xEoIs: EoI n_TOF facility upgrades, M.Bacak et al.

​

(II) s-process conditions in AGB and massive stars, first i-process nuclei

  • Measure new branching-point nuclei; extend existing data in neutron energy
    • Stations: REAR, DICER, NEAR/CYCLING, n_ACT

2xEoIs: EoI REAR, V. Alcayne et al.; EoI n_ACT, C. Lederer-Woods, A. Mengoni et al.

​

​

Programme: three physics pillars and the stations that serve them

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6

(I) Stellar models and presolar grains

  • Re-measure the stable isotopes with MACS uncertainties >5% to ≤5%
    • Stations: EAR1, EAR2, NEAR

1xEoIs: EoI n_TOF facility upgrades, M.Bacak et al.

​

(II) s-process conditions in AGB and massive stars, first i-process nuclei

  • Measure new branching-point nuclei; extend existing data in neutron energy
    • Stations: REAR, DICER, NEAR/CYCLING, n_ACT

2xEoIs: EoI REAR, V. Alcayne et al.; EoI n_ACT, C. Lederer-Woods, A. Mengoni et al.

​

(III) i- and r-process nucleosynthesis

  • First (n,γ) data on short-lived i- and r-process nuclei
    • Stations: n_ACT, ISR + neutron target

3xEoIs: EoI n_TOF facility upgrades, M.Bacak et al.; EoI n_ACT, C. Lederer-Woods, et al.; EoI ISR & Neutron Target, Y. Litvinov et al.

Programme: three physics pillars and the stations that serve them

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7

Roadmap coverage of the s-, i- and r-process paths

Adapted from M. Wiedeking et al., Nat. Rev. Phys. (2025), doi:10.1038/s42254-025-00885-7

← Pillar I →

← Pillar II →

← Pillar III →

after 20y roadmap!

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8

Courtesy of N. Liu

Pillar I · Presolar grains and stellar models need MACS to ≤5%

Presolar-grain isotope ratios are measured to a few ‰. Stellar models (AGB and massive-stars) have uncertainties of ≤5% → Nuclear data input also has to be accurate to the level of ≤5%

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9

Figure courtesy of A. Mengoni

Pillar I · Many measured MACS still exceed 5% uncertainty

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10

Only 129 of the 281 s-process isotopes in KADoNiS have MACS (kT = 30 keV) known to ≤5%. The remaining 152 are a priority of the 20-year roadmap.

Pillar I · Only 129 of 281 s-process isotopes are known to ≤5%

MACS uncertainty

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11

EAR1

EAR2

Gen.#4 Target

Pillar I · Gen.#4 target and upgraded EAR1/EAR2 to close the gap

RMS < 2%

Roadmap priority: re-measure the ~150 isotopes still above 5% MACS uncertainty (Gen.#4 target, upgraded EARs).

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12

Branching-point nuclei can be produced only in very small quantities. Existing TOF data typically cover a few % of the energy range relevant for stellar MACS (kT ≈ 5–100 keV).

Pillar II · Branching-point data cover a narrow energy range

94Nb(n,γ)

Measurements limited by:

  • in-beam backgrounds
  • neutron flux

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13

DICER concept (LANL) → CERN

Pillar II · DICER-type transmission and REAR extend the reach

REAR beamlines

Scarce samples: DICER-type binocular transmission. En range limited by γ-flash and backgrounds: REAR low-background beamline.

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14

Pillar II · Unmeasured s-process branchings within reach of REAR

A. Tarifeño-Saldivia et al., Phys. Rev. Accel. Beams (2026), doi:10.1103/5d87-m8bn

REAR beamlines

Backward extraction at REAR suppresses the γ-flash (>3× fewer prompt γ) and the high-energy neutron background, extending branching-point measurements in En.

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15

Nuclear Astrophysics priorities:

  • s-process branchings without stellar-energy data: 179Ta
  • Incomplete data or a single neutron distribution: 94Nb, 147Pm, 155Eu, 163Ho, 171Tm
  • i-process: 137Cs, 144Ce, 106Ru, 90Sr (n,γ)
  • Galactic radioactivities:
  • key production reactions of 60Fe and 182Hf via double neutron capture

Pillar II · n_ACT@BDF:

→ enables new data for s-branchings, first i-process cases and galactic radioactivities

→ world leading neutron flux in astrophysical keV range (>103 x a-NEAR flux )

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16

Adapted from M. Wiedeking et al., Nat. Rev. Phys. (2025), doi:10.1038/s42254-025-00885-7

← Pillar III →

Pillar III · i/r-process nuclei are too short-lived for targets

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17

Pillar III · Conventional TOF requires long-lived samples

neutron beam

t1/2 > yr

​

Radioactive target

>1014 atoms

n_TOF so far:

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18

Pillar III · Inverse kinematics: stored ions + neutron target

neutron beam

t1/2 > yr

​

Radioactive target

>1014 atoms

neutron target

109 n/cm2

​

n_TOF so far:

New approach:

Stored Radioactive Ion Beam

108 ions, 100 kHz, 1013 ions/s

(t1/2 = s-min-yr)

​

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19

Pillar III · Two implementation options at CERN

injection

2 GeV

PSB

​

RIB

​

Neutron

Target

compact cyclotron

R. Reifarth, Y. Litvinov et al., Phys. Rev. Accel. Beams 20, 044701 (2017); A. Tarifeño-Saldivia et al., Phys. Rev. Accel. Beams 29, 061601 (2026)

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Free-Neutron Target via spallation and 9Be(p,xn)

Phys. Rev. Accel. Beams 20, 044701 (2017)

DOI: https://doi.org/10.1103/PhysRevAccelBeams.20.044701

​

​

Phys. Rev. Accel. Beams 29, 061601 (2026)

DOI: https://doi.org/10.1103/5d87-m8bn

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21

Impact · s-, i- and r-process paths run far from stability

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22

Figures courtesy of I. Dillmann (TRIUMF)

Impact · Measured stellar (n,γ) data stay close to stability

Direct stellar-energy (n,γ) data exist almost only for stable and long-lived nuclei; the i- and r-process paths rely on theory.

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23

Figures courtesy of I. Dillmann (TRIUMF)

Impact · ISR + neutron target opens (n,γ) far from stability

​

​

ISR & Neutron Target

ISR & Neutron Target

Stored Radioactive Ion Beam

108 ions, 100 kHz, 1013 ions/s

(t1/2 = s-min-yr)

​

neutron target

109 n/cm2

​

Stored beams on a neutron target reach short-lived s-process branchings, i-process waiting points and selected r-process freeze-out nuclei.

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24

Why CERN · Neutron source, stations and ISOLDE on one site

Neutron source

PS beam on a Pb spallation target with a low duty cycle: white spectrum from meV to GeV, high instantaneous flux and high resolution

Stations

EAR1 (resolution), EAR2 (flux), NEAR (activation); n_ACT, REAR and DICER in the future

ISOLDE on site

Radioisotopically pure samples for branching points; high-intensity RIBs; a possible ISR coupled to a neutron target in the same complex

Expertise

High-accuracy cross section methodology, spallation-target design, neutron-beam collimation and RIB production: the prerequisites for the ISR concept

Track record

More than two decades of investment in the facility, detectors and trained personnel

No other facility combines all of these elements on one site.

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Run 4

LS4 / Run 5

Beyond

2028

2031

2034

2037

2041

2044

2046

Pillar 1

Precision stable

isotope measurements

(Pillar 1)

²²Ne, ⁸⁶Sr, Ba chain (EAR1)

Ca isotopic chain (EAR1+EAR2+NEAR)

Ongoing stable isotope programme: high accuracy & high resolution

sTED, STAR operational

Pillar 2-3

Radioactive

branching

points, cosmochronology, and selected i-process nuclei

¹³⁵Cs NEAR

¹³⁴Cs EAR2

107Pd EAR1/EAR2

¹⁸¹,¹⁸²Hf EAR2+n_ACT

¹³⁷Cs CYCLING

s-process branchings EAR2 + NEAR (ISOLDE) + REAR

n_ACT@BDF: s-, i-process cases [BIAS, BEAS stations]

CYCLING installed

n_ACT operational

Pillar 3

i- and r-process nuclei in inverse

kinematics

ISR full

programme

s/i/r-process

LANSCE demo spallation n-target

CRYRING demo cyclotron-driven n-target

CRYRING/TRISR early science

Experimental validation

ISR construction

ISR conceptual design + approval

Pillar 1 — stable isotopes

Pillar 2 — radioactive nuclei

Pillar 3 — inverse kinematics

Key milestone

n_ACT@BDF: s-, i-process cases [BRIS rabbit station]

ISR + Neutron Target operational

Timeline

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26

Summary

Objective

Measure the neutron-capture data needed to explain where the heavy elements come from: s-, i- and r-process

Scope

Three pillars: ~150 stable isotopes at <5%; radioactive s-branchings; short-lived i/r nuclei in inverse kinematics

Why CERN

n_TOF flux + resolution, ISOLDE samples and RIBs, n_ACT@BDF, storage-ring know-how: an ecosystem found nowhere else

Needs

Beam time; facility upgrades; n_ACT (~6 MCHF); REAR; ISR + neutron target (cost pending design)

Main challenge

Pillar III: from separate building blocks to a working ISR + neutron target, fundamental demo studies

Status

Pillars I–II ready and running into Run 4; Pillar III relies on n_Act and demonstrator phase (LANSCE, GSI)

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27

BACKUP

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28

Open questions · Example measurements

Sites and evolution

22Ne: neutron poison at low metallicity. 42–48Ca: several sites; 48Ca from supernovae or the i-process? 107Pd: galactic chemical evolution

Stellar conditions

s: 134,135Cs, 94Nb, 79Se, 147Pm, 163Ho, 171Tm, 179Ta, 205Pb. i: 137Cs, 144Ce, 90Sr, 75Ga, 80Ge, 85Br. r: 132Sn

Presolar grains and spectra

86Sr: ±10% MACS gives ~200‰ on δ(88Sr/86Sr), half the ~400‰ grain spread. 134–136Ba, 134Cs: δ(134,138Ba/136Ba). 94Nb: 94Mo in grains

Radioactivities and chronometers

181,182Hf (182Hf–182W), 205Pb (205Pb–205Tl), 107Pd (107Ag), 135Cs/133Cs in the Early Solar System. 60Fe, 182Hf via double capture at n_ACT

Beyond Pb/Bi and fission

Accurate Ns fixes the r-process residuals Nr = N⊙ − Ns. s-share of 206–208Pb, 209Bi sets the r-flow beyond Bi (next slide)

Big-Bang nucleosynthesis

7Be(n,α) and 7Be(n,p) measured at n_TOF with ISOLDE samples; full cosmological energy range at an ISR (7Be: 2.8×1010 ions/s)

Precise s-process data also test r-process yields, models and their reliability.

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s-Process branching points: still a lot to do!

s-process path (blue) with the branching point at ¹⁴⁷Nd, compared with the i-process (green) and r-process (red) paths. Figure from [2], Fig. 2.

~60

branching points can be activated along the s-process path [1, 2]

21

flagged in [1] as priority TOF targets (Käppeler et al. 2011)

Branching flow

Neutron capture competes with β-decay on nuclei with half-lives of days or more.

Stellar probes

Set by temperature, electron and neutron density: ¹³⁴Ba/¹³⁶Ba, Rb, ⁹⁶Zr, ¹⁸²Hf.

Challenge to measure

TOF and activation usually need half-lives above a few years; MACS needed to ~10%.

[1] M. Lugaro, A. Chieffi, in Astrophysics with Radioactive Isotopes, ASSL 453, Springer (2018), Ch. 12, p. 643

[2] M. Lugaro, M. Pignatari, R. Reifarth, M. Wiescher, Annu. Rev. Nucl. Part. Sci. 73, 315 (2023)

Branching points turn s-process abundances into stellar probes.

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Branching points (1/4) · From ³⁵S to ⁸⁵Kr

Isotope

T½ (lab → 300 MK)

Astrophysical relevance

n_TOF route

³⁵S

87 d

Rare ³⁶S in stars and S-rich meteorites

only ISR & NT

³⁶Cl, ⁴¹Ca

0.30 Myr; 0.10 Myr

Long-lived; ⁴¹Ca EC is T- and ρ-dependent

​

⁴⁵Ca

163 d

Rare ⁴⁶Ca in Ca-rich meteoritic material

only ISR & NT

⁵⁹Fe

44.5 d

Production of long-lived ⁶⁰Fe

n_Act (double capture on 58Fe)

⁶³Ni ★

101 yr → ≃12 yr

Rare ⁶⁴Ni and the ⁶⁵Cu/⁶³Cu ratio

​

⁶⁴Cu

12.7 h

Comparable β⁺/β⁻ rates; ⁶⁴Ni and ⁶⁵Cu

only ISR & NT

⁶⁵Zn

244 d (β⁺)

Production of ⁶⁵Cu

only ISR & NT

⁷¹Ge

11.4 d (β⁺)

Production of ⁷¹Ga

only ISR & NT

⁷⁹Se ★

0.33 Myr → ≃4 yr

Isomer gives T-dependence; ⁸¹Kr, ⁸¹Br/⁷⁹Br

Measured, EAR2

⁸⁰Br

17.7 min

β⁺/β⁻ split; production of ⁸¹Kr

only ISR & NT

⁸¹Kr ★

0.23 Myr → 2300 yr

Behaves as stable; decays to ⁸¹Br

ISR & NT

⁸⁵Kr ★

10.7 yr

Opens at Nₙ > 5×10⁸ cm⁻³; ⁸⁶Kr, ⁸⁷Rb

ISR & NT

★ Priority TOF candidates (Käppeler et al. 2011), as marked in [1] · T½ terrestrial; → value at 300 MK where given in [1]

n_TOF route: as proposed in the n_TOF post-LS4 White Book · NT = neutron target in a storage ring

[1] M. Lugaro, A. Chieffi, in Astrophysics with Radioactive Isotopes, ASSL 453, Springer (2018), Ch. 12, p. 643

⁸⁵Kr opens already at neutron densities above 5×10⁸ cm⁻³.

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Branching points (2/4) · From ⁸⁶Rb to ¹⁴³Pr

Isotope

T½ (lab → 300 MK)

Astrophysical relevance

n_TOF route

⁸⁶Rb

18.6 d

Opens at Nₙ > 10¹⁰ cm⁻³; ⁸⁷Rb, Rb in stars

only ISR & NT

⁸⁹,⁹⁰Sr, ⁹¹Y

51 d; 29 yr; 59 d

Lowers ⁹⁰,⁹¹Zr vs ⁹²Zr; Zr in SiC grains

⁸⁹Sr, ⁹¹Y: only ISR & NT

⁹³Zr

1.6 Myr

Behaves as stable; decays to ⁹³Nb

​

⁹⁵Zr ★

64 d

Opens at Nₙ > 5×10⁸ cm⁻³; ⁹⁶Zr in stars, SiC

only ISR & NT

⁹⁴,⁹⁵Nb

20 kyr → ≃9 d; 35 d

Bypasses the p-only ⁹⁴Mo

⁹⁴Nb: measured, EAR2; n_ACT; ⁹⁵Nb: only ISR & NT

⁹⁹Tc

0.21 Myr → 4.5 yr

Mostly open; ⁹⁹Ru in SiC grains

​

¹⁰⁷Pd

6.5 Myr → ≃700 yr

Behaves as stable; ¹⁰⁷Ag, ESS clock

EAR1 / EAR2

¹²⁸I

25 min

β⁺/β⁻ split; s-only ¹²⁸Xe/¹³⁰Xe

only ISR & NT

¹³³Xe

5.2 d

¹³⁴Xe; Xe-S component in SiC grains

only ISR & NT

¹³⁴⁻¹³⁷Cs ★

2.1 yr; 2.3 Myr; 13 d; 30 yr

s-only ¹³⁴Ba/¹³⁶Ba; long-lived ¹³⁵Cs (★ ¹³⁴,¹³⁵Cs)

¹³⁴: EAR2 + NEAR; ¹³⁵: NEAR; ¹³⁶: only ISR & NT; ¹³⁷: EAR2, CYCLING, n_ACT

¹⁴¹Ce

32.5 d

¹⁴²Ce, skips s-only ¹⁴²Nd

only ISR & NT

¹⁴²,¹⁴³Pr

19 h → ≃4 d; 13.6 d

Skips ¹⁴²,¹⁴³Nd; Nd isotopes

only ISR & NT

★ Priority TOF candidates (Käppeler et al. 2011), as marked in [1] · T½ terrestrial; → value at 300 MK where given in [1]

n_TOF route: as proposed in the n_TOF post-LS4 White Book · NT = neutron target in a storage ring

[1] M. Lugaro, A. Chieffi, in Astrophysics with Radioactive Isotopes, ASSL 453, Springer (2018), Ch. 12, p. 643

The Cs chain spans EAR2, NEAR, CYCLING and n_ACT.

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Branching points (3/4) · From ¹⁴⁷Nd to ¹⁷⁷Lu

Isotope

T½ (lab → 300 MK)

Astrophysical relevance

n_TOF route

¹⁴⁷Nd ★

11 d

r-only ¹⁴⁸Nd; Nd in SiC grains

only ISR & NT

¹⁴⁷,¹⁴⁸Pm ★

2.6 yr → ≃1 yr; 5.4 d

Skips ¹⁴⁷Sm, s-only ¹⁴⁸Sm; Sm in SiC

¹⁴⁷: NEAR; ¹⁴⁸: only ISR & NT

¹⁵¹Sm ★

90 yr → ≃3 yr

Strong T-dependence; ¹⁵³Eu/¹⁵¹Eu

Measured (2004)

¹⁵³Sm

46 h

¹⁵⁴Sm; ¹⁵³Eu/¹⁵¹Eu ratio

only ISR & NT

¹⁵²Eu

13.5 yr

T,ρ-dependent β±; p-only ¹⁵²Gd

​

¹⁵⁴,¹⁵⁵Eu ★

8.6 yr → ≃11 d; 4.8 yr

Gd isotopes in SiC grains

¹⁵⁵: NEAR

¹⁵³Gd ★

240 d (longer in stars)

β⁺ decay slows in stars; ¹⁵³Eu/¹⁵¹Eu

only ISR & NT

¹⁶³Dy, ¹⁶³,¹⁶⁴Ho

stable; 4.6 kyr; 29 min

¹⁶³Dy unstable in stars; s-process ¹⁶⁴Er (★ ¹⁶³Ho)

¹⁶³Ho: CYCLING, n_ACT; ¹⁶⁴Ho: only ISR & NT

¹⁶⁹Er

9.4 d

Neutron-rich ¹⁷⁰Er

only ISR & NT

¹⁷⁰,¹⁷¹Tm ★

129 d; 1.9 yr

Skips ¹⁷¹,¹⁷²Yb; Yb in SiC grains

¹⁷⁰: only ISR & NT; ¹⁷¹: n_ACT

¹⁷⁶Lu

38 Gyr (isomer 3.7 h)

Isomer coupling; s-only ¹⁷⁶Lu/¹⁷⁶Hf

​

¹⁷⁷Lu

6.6 d

Makes ¹⁷⁸Hf, lowers ¹⁷⁷Hf

only ISR & NT

★ Priority TOF candidates (Käppeler et al. 2011), as marked in [1] · T½ terrestrial; → value at 300 MK where given in [1]

n_TOF route: as proposed in the n_TOF post-LS4 White Book · NT = neutron target in a storage ring

[1] M. Lugaro, A. Chieffi, in Astrophysics with Radioactive Isotopes, ASSL 453, Springer (2018), Ch. 12, p. 643

Short-lived rare-earth branchings need ISR & NT.

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Branching points (4/4) · From ¹⁷⁹Hf to ²¹⁰Po

Isotope

T½ (lab → 300 MK)

Astrophysical relevance

n_TOF route

¹⁷⁹Hf, ¹⁷⁹,¹⁸⁰Ta

stable → ≃40 yr; 1.8 yr

Rarest nucleus ¹⁸⁰ᵐTa (★ ¹⁷⁹Ta)

¹⁷⁹Ta: CYCLING

¹⁸¹Hf

42 d

¹⁸²Hf → ¹⁸²W early Solar System clock

EAR2, n_Act

¹⁸²,¹⁸³Ta

115 d; 5.1 d

W isotopes in SiC grains

only ISR & NT

¹⁸⁵W ★

75 d

¹⁸⁶W, ¹⁸⁶Os/¹⁸⁸Os; W, Os in SiC

only ISR & NT

¹⁸⁶Re

89 h

¹⁸⁶Os, ¹⁸⁶W, ¹⁸⁷Re (Re–Os clock)

only ISR & NT

¹⁹¹Os

15 d → ≃8 d

Os isotopes in meteorites; ¹⁹³Ir

only ISR & NT

¹⁹²Ir

74 d

¹⁹³Ir; rare proton-rich ¹⁹²Pt

only ISR & NT

¹⁹³Pt

50 yr (β⁺)

Production of ¹⁹³Ir

​

²⁰⁴Tl ★

3.8 yr → ≃7 d

Strong T-dependence; s-only ²⁰⁴Pb

​

²⁰⁵Pb

17 Myr

T,ρ-dependent EC; ESS clock

EAR2 / NEAR (ISOLDE)

²¹⁰Bi

5.0 d

²¹¹Bi → ²⁰⁷Pb; end of the s process

only ISR & NT

²¹⁰Po

138 d

²¹¹Po → ²⁰⁷Pb; end of the s process

only ISR & NT

Do not open (T½ drops below days in stars): ¹⁰³Ru, ¹²³Sn, ¹²⁴Sb, ¹⁵⁶Eu, ¹⁶⁰Tb ★ (ISR & NT), ¹⁶¹Tb, ¹⁷⁵Yb, ¹⁹⁸Au, ²⁰⁵Hg

★ Priority TOF candidates (Käppeler et al. 2011), as marked in [1] · T½ terrestrial; → value at 300 MK where given in [1]

n_TOF route: as proposed in the n_TOF post-LS4 White Book · NT = neutron target in a storage ring

[1] M. Lugaro, A. Chieffi, in Astrophysics with Radioactive Isotopes, ASSL 453, Springer (2018), Ch. 12, p. 643

¹⁸¹Hf links s-process branchings to Solar System chronology.

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Scientific motivation & impact: s-process branchings

Cases for a high-flux TOF facility (FRANZ)

Unmeasurable

Partially measured / Very Challenging

Fully measured

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Unmeasurable

The i-process …

Scientific motivation & impact: i-process

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Unmeasurable

The r-process …

Scientific motivation & impact: r-process

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Why at CERN?

Component

CERN

Other facilities

RIB Facility

✅

❌ (✅)

Spallation target/expertise

✅

✅ (❌)

Storage Ring

(✅) → ISR (this EoI)

❌ (✅/❌)

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38

Resources

>40

institutes in the n_TOF Collaboration

~6 MCHF

n_ACT capital (Class 3 estimate, 3 stations)

4–5 weeks

beam per radioactive branching case at EAR2

Personnel

  • Pillar I: largely within existing Collaboration staffing
  • Pillar II: stronger ISOLDE interface; RP-trained staff for sample handling
  • Pillar III: effort with host-facility teams; dedicated ISR design & construction staff

Equipment investments

  • CYCLING transport system (LS3)
  • n_ACT@BDF: ~6 MCHF; no significant operating cost beyond capital
  • REAR: see EoI D. Cano Ott et al.
  • ISR + neutron target: cost pending technical design

Beam time & operations

  • Beam time is the main limit in Run 4–5
  • Stable isotopes: several weeks each
  • NEAR / n_ACT run parasitically: no TOF beam time
  • Facility operation largely covered by CERN institutional support

CERN-led: facility & target, n_ACT@BDF, ISR Collaboration-led: detectors, samples, analysis, personnel

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Scenarios & priorities

BASELINE

Existing areas + planned upgrades

Needs: EAR1, EAR2, NEAR, CYCLING, GEAR, Gen.#4 target

Delivers

  • Pillar I: ~150 stable isotopes towards <5%
  • Part of Pillar II: 134,135Cs, 107Pd, Hf, …
  • High-impact results through Run 5

I

II (part)

ENHANCED

+ n_ACT@BDF and REAR

Needs: n_ACT (~6 MCHF, from ~2032); REAR installed in LS4

Delivers

  • Full Pillar II: 179Ta, 94Nb, 147Pm, 163Ho, 79Se, 204Tl, …
  • First i-process cases: 137Cs, 144Ce, 90Sr
  • 60Fe production/destruction; low-background capture

I

II

III (i)

FULL AMBITION

+ ISR & neutron target

Needs: ISR at HIE-ISOLDE coupled to a free-neutron target

Delivers

  • (n,γ) on short-lived s-, i- and r-process nuclei
  • First RIB demonstration ~2040
  • Systematic programme from 2041

I

II

III

Each step is a separable package with its own EoI; the baseline already delivers Pillar I and part of Pillar II.

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Complementarity & competition

Alternatives elsewhere

n_TOF / CERN edge

Partners & complementarity

Pillar I

Stable isotopes in s-process

  • GELINA (JRC-Geel): high resolution, lower inst. flux
  • DANCE (LANSCE), J-PARC ANNRI, CSNS Back-n
  • Flux and resolution at once: small σ, small sample masses
  • Sub-5% accuracy already demonstrated
  • GELINA / DANCE for cross-checks
  • Results feed JEFF, ENDF, JENDL; NEA HPRL

Pillar II

s-branchings and first i-process

  • DANCE (high-efficiency capture)
  • Compact keV activation sources: cannot span 1 keV to several 100 keV
  • On-site ISOLDE sample production + PSI / ILL
  • NEAR/n_ACT cover the full stellar energy range (n_ACT ≈103× a-NEAR flux)
  • PSI, ILL: radioactive sample production
  • Competition limited by technical barriers

Pillar III

Inverse kinematics (short-lived i- and r-process)

  • TRISR (TRIUMF-ISAC): future parallel initiative
  • Only site combining high-intensity ISOL beams, spallation n-target expertise and low-energy storage rings
  • LANSCE, CRYRING@ESR: demonstrator partners
  • TRISR: complementary, long term

Theory is no substitute: TALYS, NON-SMOKER, SMARAGD uncertainties for branchings and i-process nuclei reach factors of 2–10, versus the ±5% stellar models need.

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Feasibility, risks & milestones

Pillar I: stable isotopes

MATURE

  • Ready: facility, detectors (C₆D₆, sTED, STAR soon), analysis frameworks
  • Limiting factor: beam time, not technology
  • Milestones: sTED/STAR and Gen.#4 target operational

Pillar II: branching points

DEMONSTRATED

  • Track record: 7 branching nuclei measured in 25 years; ISOLDE samples shown for 135Cs, 7Be
  • Needs: EAR2 optimisation, CYCLING (LS3), GEAR upgrade, approval of n_ACT / REAR / DICER
  • Milestones: n_ACT BIAS/BEAS end of Run 4; REAR commissioned 2036

Pillar III: inverse kinematics

HIGHEST RISK / RETURN

  • Status: building blocks (neutron target, low-energy storage ring, Wien-filter recoil separation) demonstrated separately
  • Main risks: full-system integration; ISR approval and funding at HIE-ISOLDE

Run 4

LANSCE spallation n-target demonstrator

Run 4

CRYRING@ESR full-system proof of principle

LS4 / Run 5

ISR conceptual design + approval

~2040

First radioactive-beam inverse-kinematics measurement

2041+

ISR full s/i/r-process programme

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Storage-Ring options for a future “production” facility

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K. Pak, B. Davids, and Y. K. Kim, Nuclear Engineering and Technology 57, 103392 (2025), arXiv:2312.11859 [physics.acc-ph].

See INTC EoI by C. Domingo-Pardo, Y. Litvinov

A. Tarifeño-Saldivia et al., Phys. Rev. Accel. Beams 29 (2026), https://doi.org/10.1103/5d87-m8bn

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Free-Neutron Target via spallation and 9Be(p,xn)

Phys. Rev. Accel. Beams 20, 044701 (2017)

DOI: https://doi.org/10.1103/PhysRevAccelBeams.20.044701

​

​

Phys. Rev. Accel. Beams 29, 061601 (2026)

DOI: https://doi.org/10.1103/5d87-m8bn

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Why at CERN? Isolde Storage Ring (ISR)

  • New ISR design by M. Grieser (2025) → This EoI
  • Including Wien-Filters for reaction product detection
  • 5.2 m experimental distance

Neutron target

Stray ions due to charge-exchange reactions with residual gas can collide only with the dipoles of the ring (not in the straight sections).

​

Catchers at the dipoles are commonly used to remove these ions, so they are not a problem, both if they are long-lived or short-lived. They can be removed easily. For radioactive beams one adds removable inserts and local shielding, so the activity can be taken out between campaigns.

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Realistic examples for neutron-capture at the ring:

η = 1e9 n/cm² → neutron density objective, both spallation/cyclotron

ISR = 1e8 ions → number of stored ions / space-charge limit ISR

f ≈ 100 kHz at ~100 keV/u → revolution frequency in the ring

I = 1e8 x 1e5 = 1e13 ions/s → particle current through the ring

Luminosity = η·I = 1e22 cm⁻²s⁻¹ → reaction luminosity

​

Reaction rate:

R = L · σ · t = 1e22 cm⁻²s⁻¹ × σ[mb] × 1e-27 cm²/mb × 24h·3600s

​

R ≈ 0.86 × σ[mb] counts/day

​

Measuring time for 10% statistical uncertainty:

​

σ = 5 mb → ~4 counts/day → ~23 days → Just one data point may be OK

σ = 10 mb → ~9 counts/day → ~12 days

σ = 50 mb → ~43 counts/day → ~2.3 days (~56 h) → Scan a few points

σ = 100 mb → ~86 counts/day → ~1.2 days (~28 h)

σ = 500 mb → ~430 counts/day → ~5.6 hours → Fully scan the CS in the energy range

​

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Summary

Goal: quantify the contributions of the s-, i- and r-processes to the heavy elements with laboratory (n,γ) data.

Three pillars

  • I · Stable isotopes: 152 of 281 s-process isotopes still have MACS uncertainties >5%; re-measure them to ≤5% at EAR1/EAR2 to interpret presolar grains and constrain AGB and massive-star models.
  • II · s-process branchings: new and extended branching-point data with REAR, DICER-type transmission and n_ACT, using samples from ISOLDE, PSI and ILL.
  • III · i- and r-process: first (n,γ) data on short-lived nuclei with NEAR-CYCLING and n_ACT, and ultimately in inverse kinematics at an ISR coupled to a neutron target.

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Summary

Why at CERN

  • White neutron spectrum (meV–GeV) from the PS and a Pb spallation target, with high instantaneous flux and high resolution.
  • Complementary stations (EAR1, EAR2, NEAR; n_ACT and REAR in the future) cover the full range of sample availability.
  • ISOLDE on site: radioisotopically pure samples, high-intensity RIBs and a possible ISR coupled to a neutron target.
  • Storage-ring and neutron-target concepts are also pursued at GSI and TRIUMF; CERN is the only site where all components are already co-located.

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