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Kinetics – �Catalysis & �Reaction Mechanisms

Lecture 9.5

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Catalysis =

- catalysts are not altered during a reaction, they serve to lower Ea and speed up the reaction by offering a different pathway for the reaction

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Catalysis

2 types of catalysts:

1) Homogeneous Catalyst =

2) Heterogeneous Catalyst =

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Reaction Mechanisms = a series of simple steps that lead the initial reactants to final products

- must be determined experimentally

- must agree with overall stoichiometry AND the experimentally determined rate law

2O3(g) 3O2(g)

Consider the following reaction:

The reaction mechanism consists of two steps:

O3(g) O2(g) + O(g)

O(g) + O3(g) 2O2(g)

2O3(g) 3O2(g)

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Reaction Mechanisms

Intermediate =

Catalyst =

Consider the following two step reaction mechanism:

H2O2(aq) + Br2(aq) 2Br-(aq) + 2H+(aq) + O2(g)

H2O2(aq) + 2Br-(aq) + 2H+(aq) Br2(aq) + 2H2O(l)

1) What are the intermediates present? Why?

2) What is the catalyst? Why?

3) What is the overall reaction?

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Reaction Mechanisms

A Products

The elementary steps may be:

Molecularity

Elementary Steps

Rate Expression

Unimolecular

Bimolecular

Termolecular

Rate = k[A]

A + B Products

Rate = k[A][B]

Rate = k[A]2

2A Products

A + B + C Products

Rate = k[A][B][C]

OR??

- the individual steps in the reaction mechanism are called elementary steps

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Reaction Mechanisms

Ex:

Step 1

Step 2

- the slow step is called the

Ex: Step 1 above

- for a reaction mechanism to be plausible, the rate expression of the RDS AND ALL STEPS PROCEEDING IT must match that of the experimentally determined rate law for the overall reaction

- in a reaction mechanism consisting of several steps, one step may be much slower than any other

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Reaction Mechanisms

1) Is this an acceptable mechanism? Justify your answer.