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Nilotpal Chakraborty – PhD student

Max Planck institute for physics of complex systems (MPIPKS), Dresden

Email: nilotpal@pks.mpg.de

Twitter: @Nilotpal_Chak

Roderich Moessner (MPIPKS) Benoit Doucot (LPTHE, Sorbonne)

arXiv:2304.13049

Riemann meets Goldstone: Magnon scattering off quantum Hall skyrmion crystals probes interplay of symmetry breaking and topology (and entanglement)

Encouraged to ask in questions

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What is a Skyrmion?

Interaction induced (in absence of Zeeman term) quantum Hall ferromagnet at 𝛎 = 1

Spin polarized state acts as a coherent source of spin waves – magnons

Cheapest charged excitations:textured spins, (Skyrmions - see fig) cheaper due to exchange – first introduced in nuclear physics in the Skyrme model

Quantum Hall setting - Sondhi et al, PRB 1993

Also occur in chiral magnets, but due to DM interaction

Skyrmions - topological excitations - quantized topological charge- also carry electric charge

S.M. Girvin – arXiv 1999

Slightly away from 𝛎 = 1 - a ground state Wigner crystal – the skyrmion crystal – Brey,Fertig,Cote and Macdonald, PRL 1995

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Magnon injection experiments

New wave of experiments which allow us to probe spin structure of ground states – a direct probe and a new paradigm of scattering experiments

Coherent source of spin waves, magnons, required – analogous to X-rays for crystals

Zhou,…..,Yacoby PNAS, 2021

Several groups

  1. Yacoby group (with Halperin) – Harvard
  2. Young group – UCSB
  3. Roulleau and Parmentier groups - Saclay

Wei et al, Science 2018

T. Zhou et al, PNAS 2021

Pierce et al, Nat. Phys. 2022

H. Zhou et al, Nat Phys. 2020

A. Assouline et al. Nat. Phys. 2021

H. Zhou et al. , PRX 2022

Experiments thus far:

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Experimental evidence for Quantum Hall Skyrmion crystals

Previous experiments fall into three types:

  1. Thermal experiments – Shayegan group, late 90s
  2. Microwave spectroscopy – Pfeiffer and West group,Bell Labs, PRL 2010
  3. NMR experiments – Above two groups and a few others

All the above mostly provide indirect evidence via spin relaxation rates/ heat capacity etc.

New platform for unambiguous evidence of crystalline order and excitation spectra – Magnon transport in Quantum Hall junctions

H. Zhou,…, A.F. Young Nat. Phys. 2020

Experiments thus far:

Wei et al, Science 2018

T. Zhou et al, PNAS 2021

Pierce et al, Nat. Phys. 2022

H. Zhou et al, Nat Phys. 2020

A. Assouline et al. Nat. Phys. 2021

H. Zhou et al. , PRX 2022

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Ferromagnet – Skyrmion crystal – Ferromagnet quantum Hall junction

FM

𝛎 = 1

FM

𝛎 = 1

SKC

𝛎 = 1 ± 𝜀

Experimental setup – “Easy experiment” – P. Roulleau, Jan 2023

Theory - Technically hard for the following reasons

  1. Need appropriate basis to interpolate between zero and finite topological charge density
  2. Can’t do naïve boundary matching- need recursive transfer matrix or Green’s functions
  3. Above approach suffers generically from fatal numerical instabilities
  4. Need to discretize topological charge density
  5. Non-linear sigma mode construction complicated by different order parameter manifolds

Inject magnon

Measure transmitted signal

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Unambiguous and direct signatures of crystalline order and excitation spectra

  1. Direct signatures for a quantum Hall skyrmion crystal phase of matter
  2. Amenable to ongoing transport experiments
  3. Uncovers excitation spectra to great detail from non-local transmission probes

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Magnon transport probes confluence of topology-symmetry breaking

Topology-symmetry breaking dichotomy results in –

  1. Riemann-Goldstone Landau level

Pinned to zero energy if one considers only exchange terms – consequence of holomorphic nature – dispersive Goldstone modes arise from this flat band

  1. Non-uniform effective Landau levels due to emergent magnetic fields

Landau level structure due to spatially modulating topological charge density of skyrmion crystal.

Direct signatures for a quantum Hall skyrmion crystal phase of matter!

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First introduced in quantum hall physics by Haldane and Rezayi (PRB 1985) for Laughlin-Jastrow wavefunctions with periodic boundaries.

Methods: 1. Basis for quantum hall junction with skyrmion crystal – Truncated theta functions

Kovrizhn, Doucot, Moessner, PRL 2013

Zeros of theta functions correspond to skyrmion cores!

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Truncated theta functions provide an analytically tractable model for ferromagnet-Skyrmion crystal-ferromagnet junctions!

Next question – how does an incoming ferromagnetic magnon scatter off of such a skyrmion lattice?

Acts as effective magnetic field – periodically modulating magnetic field with non-zero mean – possible connections to FCI physics (possible Bosonic analogue?)

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Small oscillations about minimal energy configuration – shown on earlier slide

Intuitive picture – charged particle scattering off of a region of spatially varying magnetic field

Energy functional

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How to discretize?

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Methods 2. Discretize topological charge

Nearest neighbour tight binding model!

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Methods: 3. Recursive transfer matrix approach

Tight-binding model

Transfer matrix for a slice at X

Rotate matrix to get scattering amplitudes

How to avoid numerical instabilities – At every step, instead of propagating the whole transfer matrix, propagate the reflection and transmission matrices of each slice using recursive relations from multiple scattering events

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Magnon transport probes confluence of topology-symmetry breaking

Topology-symmetry breaking dichotomy results in –

  1. Riemann-Goldstone Landau level

Pinned to E = 0 if g = 0 – holomorphic constraint – dispersive Goldstone modes arise from this flat band limit

  1. Non-uniform effective Landau levels due to emergent magnetic fields

Landau level structure due to spatially modulating topological charge density of skyrmion crystal.

Unambiguous signatures of a quantum Hall skyrmion crystal phase of matter!

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Warmup exercise – simplified model of FM/AFM/FM junction

Resolve problem of lattice mismatch

Motivation – Understand effects of kinetic mismatch and mismatch between number of goldstone modes (1 for FM, 2 for AFM)

Conventional scattering problem

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Signatures:

  1. Critical curve for incidence angle
  2. Threshold energy for transmission
  3. Sharp Fabry-Perot interference

Analysis done much better for more realistic scenarios by:

Wei, Huang, Macdonald – PRL, 2021

Atteia, Parmentier, Roulleau, Goerbig – arXiv 2022

Warmup exercise (contd.)

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Step 1- Intuitive semiclassical picture based on cyclotron orbits due to constant magnetic field

Incoming charged particle

Fully reflected

Incoming charged particle

Fully transmitted but exiting with different velocity

Assume translational invariance along y – integrable problem

Effective potential

qy -conserved

Collection of 1D modes with Veff = (qy+eAy(x))2/(2m)

Depending on x and the value of qy there are 3 types of effective potentials

Similar phenomena for a magnon scattering off of a single skyrmion in chiral magnets – skew scattering of magnons and hall effect for magnons –

Iwasaki, Beekman, Nagaosa – PRB 2014

Schutte, Garst – PRB 2014

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Energy threshold for transmission

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How do modulations of the B-field affect this picture?

 

py

x

 

Tunneling

Classically allowed trajectories

 

Characteristic signature – non-monotonic dependence of transmission coefficient on channel number!

Angular spread of transmitted signal –some angles dominant!

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Y variation introduces dispersion

X-variation pushes bands closer

Numerical results – Heuristic model

  1. Band like transmission features with sharp peaks, at energies of the bound states (Landau levels)!
  2. Multichannel interference reduces height of transmission peaks!

No transmission at all for constant B case!

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Channel non-monotonicity – periodically modulated B

Fixed incoming momenta - certain outgoing channels have majority transmission!

Angular deviation – constant B

Outgoing magnon is deflected! – similar phenomena observed in magnon scattering off single skyrmions in metallic magnets!

Consequences of crystalline order

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Lowest energy modes are pinned to zero for g = 0 – can deform spin vector in the space of holomorphic textures continuously without changing exchange energy!

Finite g induces dispersion in Goldstone modes in the Riemann-Goldstone Landau level!

Two heuristic models capture most qualitative physics

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What about anisotropies?

Our model – isotropic SU(2) skyrmion crystal – 4 goldstone modes – 3 SU(2) generators + 1 for broken translational invariance

Anisotropies (such as a zeeman term) will gap out some of the goldstone modes, but probably not all (see R. Cote et al. PRB 2007).

Hence some signatures should remain, however, signatures of higher effective landau levels should be robust.

Cote et al, PRB 2007

Several anisotropies present in actual experiment – zeeman term, lattice scale anisotropie etc.

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Outlook

Experiment - Unambiguous determination of the presence of a quantum Hall skyrmion crystal from magnon transport – such signatures are absent in any other possible competing phase in the quantum Hall phase diagram. Unveils the excitatioin spectrum to great detail.

Theory – Skyrmion crystal provides a fertile platform to probe the intersection of topology anf symmetry breaking which manifests in rich physics, c.f – Riemann Goldstone Landau level. Interaction of spin waves from collinear ferromagnets with non-collinear spinn structures such as skyrmion crystals - techniques transferrable to other settings such as chiral magnets, or situations with artificial gauge fields

Next step – SU(4) skyrmion crystals, especially configurations where spin and valley degrees of freedom are entangled (“Entanglement skyrmions” – Doucot, Goerbig, et al. PRB 2008)

Can one detect spin-valley entanglement from magnon transport signatures?

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Spin-valley entanglement skyrmions – Mulitcomponent quantum Hall

X

Variational wavefunction at 𝛎 = 1

Coulomb interaction- approximate SU(4) symmetry (2 spin + 2 valley)

Schmidt decomposition of CP3 spinor – natural way to express entanglement

6 real parameters

 

Maximally entangled

Doucot et al, PRB 2008, Lian and Goerbig – PRB 2017

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Spin and pseudospin vector vanishes at maximal entanglement!

Visualize via three Bloch spheres – Spin, Pseudospin and Entanglement

Doucot et al, PRB 2008, Lian and Goerbig – PRB 2017

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Skyrmion crystal minimization problem – optimal textured configuration in presence of anisotropies

Question – Analytic ansatz for CP3 skyrmion crystals?

Use basis of four theta functions – p = 0,1,2,3

Interesting method question – How to construct an appropriate parametrization of an SU(4) matrix (in the basis of theta functions), whose first column is fixed?

Answer comes from Random Matrix theory literature

Result – a random 4*4 SU(4) matrix with 9 Euler angles

Minimize F over the integral of EA over the entire slab

Topological charge density much smoother than SU(2)

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Strips of vanishing magnitude of spin vector!

Optimal configuration in presence of anisotropies

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Strips of maximal entanglement – entanglement skyrmion crystal

Maximal entanglement – magnitude of spin vector vanishes along strips – maximal mismatch with incoming magnon

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THANK YOU!

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Summary

Magnon transport in quantum Hall heterojunctions in graphene -

  1. Novel way to detect spin structure in quantum Hall phases

First direct signatures of a skyrmion crystal!

  1. New class of scattering problems between topologically trivial and non-trivial (induced by spin/pseudospin) junctions

Topology-symmetry breaking dichotomy in skyrmion crystal results in:

  1. Riemann-Goldstone Landau level
  2. Non-uniform effective higher Landau levels due to emergent magnetic fields (Not the externally applied one)

Magnon transport in such junction like setups allows one to probe crystalline order, dispersion and number of Goldstone modes, and width of higher Landau levels!

  1. Spin-valley entanglement natural in graphene
  2. Possibility of entangled skyrmion crystals
  3. Regions of maximal entanglement provide maximum mismatch for magnon transport – expect distinct non-local transmission signatures “quantifying” entanglement

Email: nilotpal@pks.mpg.de

Twitter: @Nilotpal_Chak

arXiv:2304.13049