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Water Treatment

Summary: The point of this lesson is to introduce students to a conventional method for treating contaminated water. Students will become more aware of drinking water sources, common types of contaminants in source water, and treatment using coagulation/sedimentation. They will also consider how particle size relates to surface area, as well as how the charges of metal oxide nanoparticle surfaces and contaminants are essential for explaining how they interact with one another during the treatment process.

Nanoscience Connection: Coagulation and sedimentation is widely used for water treatment because it is relatively cheap and effective at removing a variety of contaminants. The process involves formation of nanosized iron and/or aluminum hydroxides that react with contaminants through surface adsorption and other processes. The properties of nanoparticle surfaces including area, charge, reactivity, and adsorption are key concepts in nanoscience and nanotechnology. By learning about conventional water treatment, students are ready to understand alternative treatment strategies, as well as how contaminants interact with nanoparticles in environmental systems e.g., soils.

Learning Objectives:

  • Give examples of common drinking water sources and types of contaminants
  • Describe conventional water treatment using coagulation and sedimentation
  • Describe the relationship between nanoparticle size and surface area
  • Explain how the surfaces of a particle are charged in water
  • Define adsorption and explain the role it plays in conventional water treatment

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Water Treatment

Key Concepts:

  • Drinking Water Sources & Contaminants
    • Nanoparticle Size vs. Surface Area
    • Surface Charge & Reactivity
    • Adsorption

Google images

Module: Environmental Nanoscience

2022 Nanoscience Professional Development Workshop

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What is the original source of the drinking water in your area?

  • Shallow groundwater wells
  • Deep groundwater wells
  • Artesian springs
  • Glacial meltwaters
  • Reservoirs or lakes
  • Rivers or streams

Where does the water from your tap come from?

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Surface Water Sources

Streams, Rivers, Lakes, Reservoirs

The New River

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Credit: ReNew the New – Regional New River Cleanup

Surface Water Sources

Streams, Rivers, Lakes, Reservoirs

The New River

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Credit: ReNew the New – Regional New River Cleanup

Surface Water Sources

Streams, Rivers, Lakes, Reservoirs

Cleanwisconsin.org

The New River

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What types of natural and anthropogenic contaminants are common in raw source water?

Credit: www.blacksburg.gov

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What types of natural and anthropogenic contaminants are common in raw source water?

  • Microbial:Viruses, bacteria can come from sewage treatment plants, septic systems, agricultural livestock operations, or wildlife

Credit: www.blacksburg.gov

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What types of natural and anthropogenic contaminants are common in raw source water?

  • Microbial:Viruses, bacteria can come from sewage treatment plants, septic systems, agricultural livestock operations, or wildlife
  • Inorganic:Salts and metals, naturally occurring or result from urban storm-water runoff, industrial or domestic wastewater discharges, mining, or farming

Credit: www.blacksburg.gov

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What types of natural and anthropogenic contaminants are common in raw source water?

  • Microbial:Viruses, bacteria can come from sewage treatment plants, septic systems, agricultural livestock operations, or wildlife
  • Inorganic:Salts and metals, naturally occurring or result from urban storm-water runoff, industrial or domestic wastewater discharges, mining, or farming
  • Pesticides & Herbicides: Sources such as agriculture, urban storm-water runoff, and residential uses

Credit: www.blacksburg.gov

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What types of natural and anthropogenic contaminants are common in raw source water?

  • Microbial:Viruses, bacteria can come from sewage treatment plants, septic systems, agricultural livestock operations, or wildlife
  • Inorganic:Salts and metals, naturally occurring or result from urban storm-water runoff, industrial or domestic wastewater discharges, mining, or farming
  • Pesticides & Herbicides: Sources such as agriculture, urban storm-water runoff, and residential uses
  • Organic Chemical: Synthetic and volatile organics, by-products of industrial processes and petroleum production, gas stations, storm-water runoff, and septic systems

Credit: www.blacksburg.gov

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What types of natural and anthropogenic contaminants are common in raw source water?

  • Microbial:Viruses, bacteria can come from sewage treatment plants, septic systems, agricultural livestock operations, or wildlife
  • Inorganic:Salts and metals, naturally occurring or result from urban storm-water runoff, industrial or domestic wastewater discharges, mining, or farming
  • Pesticides & Herbicides: Sources such as agriculture, urban storm-water runoff, and residential uses
  • Organic Chemical: Synthetic and volatile organics, by-products of industrial processes and petroleum production, gas stations, storm-water runoff, and septic systems
  • Radioactive: Naturally occurring or result of oil and gas production and mining activities

Credit: www.blacksburg.gov

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Dissolved vs. Solids

Credit: Western Oregon University

Sodium Chloride

SOLID PARTICLES

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Dissolved vs. Solids

Credit: Western Oregon University

Sodium Chloride

SOLID PARTICLES

Sodium Chloride

DISSOLVED IONS

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Size Classification of Contaminants

Credit: Maarten Bloemen

water

DISSOLVED IONS

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Size Classification of Contaminants

Credit: Maarten Bloemen

water

CLAY

SILT

SAND

GRAVEL

DISSOLVED IONS

SOIL PARTICULATES

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Size Classification of Contaminants

Credit: Maarten Bloemen

water

CLAY

SILT

SAND

GRAVEL

DISSOLVED IONS

SOIL PARTICULATES

What methods are there to remove contaminants that vary so widely in size?

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Filtration

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Filtration

Challenges:

  • Typical pore sizes (e.g., 0.2 μm or larger) do not capture dissolved contaminants
  • Smaller pore sizes have slower flow, easier to plug
  • Filtration is $$$ (maintenance, consumables, waste, etc.)

Credit: Wikipedia

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How is source water made safe for consumption?

?

Credit: Google images

A common treatment method is deactivating contaminants by surface adsorption

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How is source water made safe for consumption?

Credit: Google images

A common treatment method is deactivating contaminants by surface adsorption

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Conventional Water Treatment

Example: The New River

New River

Blacksburg, VA

NRV Regional Water Authority

Credit: www.blacksburg.gov

Credit: Google maps

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http://www.blacksburg.gov/

NRV Regional Water Authority

Total capacity ~12.5 million gallons/day

Credit: Google maps

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Conventional Water Treatment �is a multi-stage process that removes dissolved and particulate contaminants and disinfects source water

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Conventional Water Treatment �is a multi-stage process that removes dissolved and particulate contaminants and disinfects source water

  • Coagulation: Aluminum or iron salts are mixed with source water and precipitate as nanosized particles that are positively charged

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Conventional Water Treatment �is a multi-stage process that removes dissolved and particulate contaminants and disinfects source water

  • Coagulation: Aluminum or iron salts are mixed with source water and precipitate as nanosized particles that are positively charged
  • Sedimentation: Particles come out of suspension (flocculation), grow (coalescence), and settle due to gravity

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Credit: www.safewater.org

Small particles take longer to settle than larger particles.

Increasing particle size through aggregation and growth speeds up the process.

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Big particle

Medium particles same overall size 20x more surface area

Tiny particles same overall size 60x more surface area

Nanoparticle Size vs. Surface Area

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Big particle

Medium particles same overall size 20x more surface area

Tiny particles same overall size 60x more surface area

Nanoparticle Size vs. Surface Area

  • Surface area increases with decreasing particle size

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Big particle

Medium particles same overall size 20x more surface area

Tiny particles same overall size 60x more surface area

Nanoparticle Size vs. Surface Area

  • Surface area increases with decreasing particle size
  • Surfaces atoms important for chemical reactions

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Phase

Surface Area (m2/g)

Site Density (per nm2)

Ferric hydroxides

Up to 500

2-20

Aluminum hydroxides

Up to 150

2-12

One (1) gram of material can have more surface area than a full-size basketball court!

Credit: Good Food Grower

Credit: Virginia Tech

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Surface Chemistry

Metal oxide surfaces are amphoteric: can react both as an acid or base (+ or -)

Schematic representation of the distribution of positive, negative, and neutral surface hydroxyl groups on an iron oxide surface

Image Credit: The Iron Oxides by Cornell & Schwertmann. © 2003 Wiley-VCH

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Surface Chemistry

Metal oxide surfaces are amphoteric: can react both as an acid or base (+ or -)

Schematic representation of the distribution of positive, negative, and neutral surface hydroxyl groups on an iron oxide surface

Image Credit: The Iron Oxides by Cornell & Schwertmann. © 2003 Wiley-VCH

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Surface Chemistry

Metal oxide surfaces are amphoteric: can react both as an acid or base (+ or -)

Schematic representation of the distribution of positive, negative, and neutral surface hydroxyl groups on an iron oxide surface

Image Credit: The Iron Oxides by Cornell & Schwertmann. © 2003 Wiley-VCH

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Surface Chemistry

Metal oxide surfaces are amphoteric: can react both as an acid or base (+ or -)

Image Credit: The Iron Oxides by Cornell & Schwertmann. © 2003 Wiley-VCH

Schematic representation of the distribution of positive, negative, and neutral surface hydroxyl groups on an iron oxide surface

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Zeta potential (ζ) refers to the electrical charge at the surface of the hydrodynamic shear layer surrounding a particle.

Image Credit: Science Direct

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Neutral

Surface Charge

pH determines whether the net surface charges of particles can be negative, positive, or neutral (zero)

Image Credit: Wiese & Healy (1975) J. Colloid Interface Sci. 51, 427

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Surface Charge

+

Neutral

Surface Charge

pH determines whether the net surface charges of particles can be negative, positive, or neutral (zero)

Image Credit: Wiese & Healy (1975) J. Colloid Interface Sci. 51, 427

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Surface Charge

+

Neutral

pH Point of Zero Charge

Surface Charge

pH determines whether the net surface charges of particles can be negative, positive, or neutral (zero)

Image Credit: Wiese & Healy (1975) J. Colloid Interface Sci. 51, 427

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Mineral Surfaces

Mineral Surfaces

AsO43-, PO43-, SO42-, NO3-

Organic molecules

Transition metals �e.g., Cr(H2O)63+

Complex cations �e.g., uranyl UO22+

Opposites Attract!

Dissolved species, molecules, and particles interact due to similarities and differences in net charges

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Mineral Surfaces

Mineral Surfaces

AsO43-, PO43-, SO42-, NO3-

Organic molecules

Transition metals �e.g., Cr(H2O)63+

Complex cations �e.g., uranyl UO22+

Opposites Attract!

Dissolved species, molecules, and particles interact due to similarities and differences in net charges

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Adsorption vs. Absorption

In chemistry, absorption is the diffusion of particles of gas or liquid into a material (e.g., water into a sponge)

Google images

Shutterstock

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Adsorption

Separation of a substance from one phase accompanied by its accumulation or concentration at the surface of another

Mineral

Outer-sphere complex

weaker, electrostatic attraction (hydrogen bonding important)

Inner-sphere complex

Strong, bonded directly to surface (bridging oxygens)

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Adsorption

Separation of a substance from one phase accompanied by its accumulation or concentration at the surface of another

Mineral

Outer-sphere complex

Weak, electrostatic attraction (hydrogen bonding important)

Inner-sphere complex

Strong, bonded directly to surface (bridging oxygens)

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Adsorption

Separation of a substance from one phase accompanied by its accumulation or concentration at the surface of another

Mineral

Outer-sphere complex

Weak, electrostatic attraction (hydrogen bonding important)

Inner-sphere complex

Strong, bonded directly to surface (bridging oxygens)

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Credit: Genesis Water Technologies

Conventional Water Treatment

Coagulation/flocculation & sedimentation remove a majority of organic and inorganic contaminants, but not all…

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Anthracite coal

Fine sand

Coarse sand �& stone

Filtration

Removes remaining flocs, algae, and dissolved cations

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Key Takeaways…

  • Coagulation & sedimentation is a relatively cheap and efficient way to treat drinking water
  • Large amount of highly reactive and charged surfaces drives interactions between dissolved species (ions and molecules) and other particles
  • Adsorption to nanoparticle surfaces immobilizes and deactivates contaminants
  • Processes critical to water treatment methods and movement and cycling of elements in the environment