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Intense Laser Induced Nuclear Polarization

Han-Xu Zhang

zhanghanxu@fudan.edu.cn

Taiyuan · Shanxi IWND2026

2026.08.23

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  1. Background
  2. Highly nonlinear light-nucleus interaction
  3. Intense laser induced nuclear polarization
  4. Discussions and prospects

CONTENTS

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Background

Intense Laser Induced Nuclear Polarization

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Background

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1896

Becquerel discover radioactivity

1909

Rutherford discover nucleus

1932

Chadwick discover neutron

1939

Hahn discover nuclear fission

1942

Fermi establish

chain reactor

Radioactivity

Nuclear fission

Nuclear fusion

Energy, agriculture, industry, healthcare …

Nuclear transition

battery, laser, clock …

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Background

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LARGE

SHORT

MULTIPOLE

 

DIFFICULT!

 

 

…

 

 

 

 

…

 

 

 

 

Bremsstrahlung

Nonlinear Compton scattering

XFEL

new possibilities?

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Background

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…

 

 

 

 

…

 

 

 

 

Transition moment

Interaction energy

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Strong field atomic physics

Attosecond science

Not enough for nuclear system

 

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Background

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…

 

 

 

 

…

 

 

 

 

+

 

 

 

…

…

 

…

…

 

 

= hyperfine

structure

Hyperfine splitting is within the reach of super intense laser!

Highly charged ion + intense laser = novel nuclear manipulation

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Background

8

 

nuclear

excitation

high harmonic

generation

Phys. Rev. Lett. 133, 152503 (2024)

Phys. Rev. C 111, 044614 (2025)

T. Li, H. X. Zhang and X. Wang, in preparation

Phys. Rev. C 113, 044315 (2026)

Highly charged ion + intense laser = novel nuclear manipulation

 

 

 

 

 

 

…

…

H. X. Zhang, T. Li, and X. Wang, under review

H. X. Zhang, B. S. Tu, X. Wang, and Y. G. Ma, in preparation

Efficient and more general way to polarize nuclear / heavy ion quantum state

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Highly nonlinear �light-nucleus interaction

Intense Laser Induced Nuclear Polarization

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Highly nonlinear light-nucleus interaction

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time-dependent Schrödinger / Dirac equation

excitation probability

 

 

qualitative measure of the strength of the light–matter interaction

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Highly nonlinear light-nucleus interaction

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excitation probability

 

 

Laser duration = 100 a.u.

 

 

vs.

 

efficient excitation

non-resonant excitation: RWA not valid & no analytical solution

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Highly nonlinear light-nucleus interaction

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…

…

 

circularly polarized laser

&

a sequence of lasers?

…

…

CP pulses

Highly charged ions

Ground state distribution

 

 

 

 

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Intense laser induced nuclear polarization

Intense Laser Induced Nuclear Polarization

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Intense laser induced nuclear polarization

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1st pulse

~100 fs

uniformly distributed in the ground state

radiative decay

0.1-100 ms

2nd pulse

radiative decay

cycle 1

cycle 2

cycle

3,4,...

polarized distribution

start

 

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Intense laser induced nuclear polarization

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H. X. Zhang, T. Li, and X. Wang, under review.

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Intense laser induced nuclear polarization

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H. X. Zhang, B. S. Tu, X. Wang, and Y. G. Ma, in preparation

Multi-pulses: achieve 100%

 

 

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Intense laser induced nuclear polarization

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H. X. Zhang, T. Li, and X. Wang, under review.

BRUTE FORCE !

Applicable to more highly charged heavy ion considered here

 

 

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Intense laser induced nuclear polarization

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Extend to other nuclei

 

H. X. Zhang, B. S. Tu, X. Wang, and Y. G. Ma, in preparation

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Discussions �and prospects

Intense Laser Induced Nuclear Polarization

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Discussions

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Existing methods

Dynamic nuclear polarization

microwave

 

 

spontaneous emission

 

Optical pumping

Resonant pumping + spontaneous emission cycles

  • NMR, MRI
  • Bioimaging
  • Polarized target
  • Commercialized
  • Light nuclei, solid host
  • resonant

 

  • SEOP, MEOP for He-3, Xe-131
  • Clock, MRI ……

Our method is the highly nonlinear, non resonant version of optical pumping

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Prospects

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super intense laser

  • Brute force
  • Short time interaction (within ps)

highly charged heavy ion

  • Sufficiently deep Coulomb potential
  • Stable unpaired electron

Ionization energy of the 1s electron in H-like thorium-229: 125 keV

Potential experimental facilities

  • Ion traps (EBIT, Penning Trap)
  • HCI production and storage
  • Shanghai Penning Trap @ FDU

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  • Ion storage ring + lasers, PHELIX @ GSI
  • HIAF @ IMPCAS

Potential applications

  • Precision measurement
  • Initial state preparation for heavy ion collision
  • ……

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Thanks

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Prof. Yu-Gang Ma @ ECNU & FDU

Prof. Xu Wang @ GSCAEP

Prof. Bing-Sheng Tu @ FDU

Dr. Tao Li @ CUHK

Thanks for your attention!

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Thanks